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Modeling the effects of reduced permeability on the photochemical reactivity of chromophoric dissolved organic matter in the open ocean.
Reduced oxy-anions of organic compounds have been observed and quantified in some open ocean mesocosms and laboratory microcosms. These anions appear to decrease the photochemical reactivity of the parent species. We sought to better understand these effects by modeling the rates of photochemical reactions of a representative organic compound (phenol) that is subject to attenuation in the ocean. The model employed was structured to mirror that of three mesocosm experiments with reduced oxy-anion concentrations. The model incorporates a cascade of reactions that begins with the photolysis of the parent and stops upon reaching equilibrium. Without photolysis, the model predicts a 5-fold reduction in reaction rates relative to the ambient conditions. The addition of reduced oxy-anions to the model increases the half-time for the reaction by a factor of 10, indicating that the oxy-anions are acting as a large mass sink for the